I do a little bit of video stuff, but I'm unclear what you are actually asking?
If you want your VLC player to play your video files, you do not need to "move" them. Just open them with the player.
You can browse to the video files, right click and click on "open with" then select your VLC player and put a checkmark where it says to always open that file type using that program.
If you are only wanting a player that will basically play any video type, just install the free k-lite codec pack for windows media player and then it will play pretty much anything except .mov files, which are mac files and played using quicktime.
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